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- W4313237951 abstract "Hydrogels are three-dimensional networks of hydrophilic polymers that have garnered significant attention as wound-healing materials. Many synthetic hydrogels are fabricated using a radical polymerization approach that requires an initiator molecule that is often photo- or thermosensitive. Initiator-free hydrogels are an emerging area of research that focuses on hydrogel fabrication that occurs in the absence of an initiator or cross-linker molecule, making these hydrogels highly relevant in tissue engineering and regenerative medicine due to their excellent cytocompatibility and ease of scale-up. Here we present on the development of initiator-free zwitterionic hydrogels that photopolymerize without any initiator or cross-linker while under cytocompatible conditions. The hydrogels exhibit a wide range of mechanical characteristics that are dependent on their polymer composition. They resist nonspecific protein adsorption and exhibit a sustained release of proteins and small molecules. Additionally, these self-initiated hydrogels significantly mitigate inflammatory macrophage activation in vitro. Overall, the development of self-initiated photopolymerized zwitterionic hydrogels offers significant progress in the fields of biomaterials and materials science." @default.
- W4313237951 created "2023-01-06" @default.
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- W4313237951 date "2022-12-27" @default.
- W4313237951 modified "2023-09-27" @default.
- W4313237951 title "Self-Initiated Photopolymerization of Anti-Inflammatory Zwitterionic Hydrogels with Sustained Release" @default.
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- W4313237951 doi "https://doi.org/10.1021/acsmacrolett.2c00713" @default.
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