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- W4313252364 abstract "Lithium (Li) metal is a promising material for high-energy–density batteries, but it is still plagued by obvious capacity degradation and low average Coulombic efficiency resulting from dendrite Li propagation. One main reason is the electro-mechanic coupled failure of plated Li on the current collector, which contributes to non-dense Li deposition on the anode. Transition metal oxides (TMOs) with a conversion-type mechanism have been used directly as the anode materials for lithium ion batteries, which demonstrated better electro-mechanical stability than metal Li. Herein, a successive ''conversion-deposition'' mechanism is ingeniously developed to restrain the generation of dendritic Li. Specifically, a micro-crystalline Cu2O modified current collector was prepared, in which Li+ are sequentially inserted into Cu2O and deposited in the form of Li metal at successive low potential. A Li-Cu half-cell based on the hybrid mechanism sustains a high Coulombic efficiency of over 99.3 % in up to 800 cycles. This work ingeniously inhibits the generation of dendrite Li by incorporating conversion-type materials with deposition-dissolution type metal Li, which contributes to a novel concept for the design of functional current collectors for composite Li anodes." @default.
- W4313252364 created "2023-01-06" @default.
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- W4313252364 date "2023-04-01" @default.
- W4313252364 modified "2023-10-16" @default.
- W4313252364 title "A successive “conversion-deposition” mechanism achieved by micro-crystalline Cu2O modified current collector for composite lithium anode" @default.
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- W4313252364 doi "https://doi.org/10.1016/j.jiec.2022.12.035" @default.
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