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• W4313253642 abstract "Carbon-based zinc-ion capacitors (ZICs) have sparked intense research enthusiasm because of large power density, good rate capability and cycling stability. However, there is still a long way to go before they achieve commercial applications. Herein, oxygen-enriched lignin-derived porous carbon nanosheets (OLCKs) were prepared by one-step carbonization-activation method, and more O-containing functional groups were generated on the surface of the porous carbon by post-surface functionalization strategy. The self-doped N can change the electron distribution of carbon skeleton and decrease energy barrier of chemical absorption of Zn2+/H+. Meanwhile, the carbonyl group can significantly enhance the wettability of OLCKs. Furthermore, the diffusion-controlled reactions mainly exist at high and low potential ranges in CV curves, which demonstrates the occurred Faradaic reaction. Consequently, the assembled aqueous ZICs based on OLCKs demonstrate a capacity of 121.7 mAh/g at 0.3 A/g, energy density of 94.3 Wh kg-1 and good cyclic stability. Besides, the assembled Zn//PVA/LiCl/ZnCl2(gel)//OLCK4 ZIC can also achieve energy density of 134.4 Wh kg-1 at 0.1 A/g. This work provides a novel design strategy by incorporating abundant O and N-containing functional groups to enhance energy density." @default.
• W4313253642 created "2023-01-06" @default.
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• W4313253642 date "2023-04-01" @default.
• W4313253642 modified "2023-10-18" @default.
• W4313253642 title "Oxygen-enriched lignin-derived porous carbon nanosheets promote Zn2+ storage" @default.
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• W4313253642 doi "https://doi.org/10.1016/j.jcis.2022.12.069" @default.
• W4313253642 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36577358" @default.
• W4313253642 hasPublicationYear "2023" @default.
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