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- W4313256213 abstract "Three-component enantioselective alkenylation of organophosphonates via nickel metallaphotoredox catalysisLi et al.ChemOctober 14, 2022In BriefHerein, we report a metallaphotoredox-catalyzed asymmetric three-component method to access a diverse array of enantio-enriched α-alkenyl phosphonates from readily available vinyl phosphonates, alkenyl halides, and alkyl trifluoroborates under mild conditions. This operationally simple and redox-neutral protocol exhibits a broad substrate scope and excellent chemo-, regio-, stereo-, and enantioselectivity. Detailed computational and experimental studies were undertaken to elucidate the mechanism and origin of the observed reactivity and selectivity. Full-Text PDF" @default.
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- W4313256213 date "2023-01-01" @default.
- W4313256213 modified "2023-09-29" @default.
- W4313256213 title "Computational methods in unraveling the mechanism of metallaphotoredox catalysis" @default.
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- W4313256213 doi "https://doi.org/10.1016/j.chempr.2022.12.011" @default.
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