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• W4313261746 abstract "The anaerobic fermentation gas (AFG) with CO2 removed is a sustainable energy resource, and converting CO2 in AFG to value-added chemicals can kill two birds with one stone. Herein, an ionic porous organic polymer (IPOP-3) catalyst, with triply synergistic effect of its hydroxide anions, nitrogen activation sites and porous structure, is synthesized. IPOP-3 exhibits an excellent ability to enrich and convert 50 vol.% CO2 by the reactions with various amines into corresponding formamides. The catalyst is also successfully applied to the N-formylation of CO2 in AFG, and can be easily recovered and reused. The plausible mechanism for the catalytic N-formylation is proposed. The hydroxide anion in IPOP-3 activates the Si−H bond of phenyl silane which reacts with the captured CO2 to form formate anion to facilitate the subsequent conversion into formamide. Our work provides a new idea for the purification of AFG and the resource utilization of CO2." @default.
• W4313261746 created "2023-01-06" @default.
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• W4313261746 date "2023-01-23" @default.
• W4313261746 modified "2023-10-18" @default.
• W4313261746 title "Effective <i>N</i> ‐formylation of Amines with CO ₂ in Anaerobic Fermentation Gas Catalyzed by Triply Synergistic Effect of Ionic Porous Organic Polymer" @default.
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• W4313261746 doi "https://doi.org/10.1002/cctc.202201351" @default.
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