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- W4313269118 abstract "Polyaromatic hydrocarbons (PHAs) containing heteroatoms have attracted considerable attention due to their potential utility in electronic devices. This work reported a novel domino reaction between an aryne precursor and azadiene bearing a benzothiophene moiety to produce a series of PHAs containing sulfur and nitrogen atoms. Further transformation of the product enabled concise synthesis of a new AIEgen, whose photophysical properties were characterized. Density functional calculations on the reaction mechanism revealed that the in situ generated aryne could trigger either a [4 + 2] or [3 + 2] process with azadiene, in which the regioselectivity was mainly a result of the heteroatom effect and may be understood by means of Houk's distortion-interaction model." @default.
- W4313269118 created "2023-01-06" @default.
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- W4313269118 date "2022-12-29" @default.
- W4313269118 modified "2023-10-18" @default.
- W4313269118 title "Construction of Polyaromatic Hydrocarbons Containing Sulfur and Nitrogen via Controllable Domino Reactions and DFT Studies" @default.
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- W4313269118 doi "https://doi.org/10.1021/acs.orglett.2c03958" @default.
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