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- W4313311919 abstract "Lithium-rich antiperovskites (LiRAPs) solid electrolytes have attracted extensive interest due to their advantages of structural tunability, mechanical flexibility, and low cost. However, LiRAPs are instinctively hygroscopic and suffer from decomposition in air, which not only diversifies their electrochemical performances in present reports but also hinders their application in all-solid-state lithium batteries (ASSLBs). Herein, the origin of the hygroscopicity, and also the effect of the hygroscopicity on the electrochemical performances of Li3-x (OHx )Cl are systematically investigated. Li3-x (OHx )Cl is demonstrated to be unstable in the air and prone to decompose into LiOH and LiCl. Nevertheless, with fluorine doping on chlorine sites, the hygroscopicity of LiRAPs is suppressed by weakening the intermolecular hydrogen bond between LiRAPs and H2 O, forming a moisture-resistive Li3-x (OHx )Cl0.9 F0.1 . Taking advantage of its low melting point (274 °C), two prototypes of ASSLBs are assembled in the ambient air by means of co-coating sintering and melt-infiltration. With LiRAPs as the solder, low-temperature sintering of the ASSLBs with low interfacial resistance is demonstrated as feasible. The understanding of the hygroscopic behavior of LiRAPs and the integration of the moisture-resistive LiRAPs with ASSLBs provide an effective way toward the fabrication of the ASSLBs." @default.
- W4313311919 created "2023-01-06" @default.
- W4313311919 creator A5011241874 @default.
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- W4313311919 date "2023-02-08" @default.
- W4313311919 modified "2023-10-12" @default.
- W4313311919 title "Enhanced Moisture Stability of Lithium‐Rich Antiperovskites for Sustainable All‐Solid‐State Lithium Batteries" @default.
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- W4313311919 doi "https://doi.org/10.1002/adma.202210365" @default.
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