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- W4313311937 abstract "The effect of the density of active molecules in molecular junctions (MJs) has been investigated by using a host/guest strategy. Mixed layers consisting of oligothiophene (BTB) encapsulated by β-cyclodextrin (BTB@β-CD) were generated. Cyclodextrins were then removed, and the pinholes generated were filled with BTB to obtain BTB@BTB films. MJs based on mixed BTB@β-CD and BTB@BTB layers, as well as single-component BTB MJs, were compared. The variation of ln J vs thickness is similar for all systems while the Jo of BTB@β-CD MJs is 20 times lower than that of BTB MJs. After β-cyclodextrin has been removed, and the pinholes filled, Jo increases and reaches the same value as for the BTB MJs, showing that the conductance scales with the number of active molecules. This strategy provides a unique method for investigating molecular interactions in direct tunneling MJs as well as the possibility of fabricating new functionalized MJs based on mixed layers." @default.
- W4313311937 created "2023-01-06" @default.
- W4313311937 creator A5030686406 @default.
- W4313311937 creator A5052368461 @default.
- W4313311937 creator A5055044328 @default.
- W4313311937 date "2022-12-20" @default.
- W4313311937 modified "2023-09-30" @default.
- W4313311937 title "Probing the Effect of the Density of Active Molecules in Large-Area Molecular Junctions" @default.
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- W4313311937 doi "https://doi.org/10.1021/acs.jpclett.2c03027" @default.
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