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- W4313313087 abstract "Abstract Boosting charge separation and transfer of photoanodes is crucial for providing high viability of photoelectrochemical hydrogen (H 2 ) generation. Here, a structural engineering strategy is designed and synthesized for uniformly coating an ultrathin CoFe bimetal‐organic framework (CoFe MOF) layer over a BiVO 4 photoanode for boosted charge separation and transfer. The photocurrent density of the optimized BiVO 4 /CoFe MOF(NA) photoanode reaches a value of 3.92 mA cm −2 at 1.23 V versus reversible hydrogen electrode (RHE), up to 6.03 times that of pristine BiVO 4 , due to the greatly increased efficiency of charge transfer and separation. In addition, this photoanode records one onset potential that is considerably shifted negatively when compared to BiVO 4 . Transient absorption spectroscopy reveals that the CoFe MOF(NA) prolongs charge recombination lifetime by blocking the hole‐transfer pathway from the BiVO 4 to its surface trap states. This work sheds light on boosting charge separation and transfer through structural engineering to enhance the photocurrent of photoanodes for solar H 2 production." @default.
- W4313313087 created "2023-01-06" @default.
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- W4313313087 date "2022-12-29" @default.
- W4313313087 modified "2023-10-13" @default.
- W4313313087 title "Structural Engineering of BiVO<sub>4</sub>/CoFe MOF Heterostructures Boosting Charge Transfer for Efficient Photoelectrochemical Water Splitting" @default.
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- W4313313087 doi "https://doi.org/10.1002/smll.202205246" @default.
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