Matches in SemOpenAlex for { <https://semopenalex.org/work/W4313331271> ?p ?o ?g. }
- W4313331271 endingPage "3415" @default.
- W4313331271 startingPage "3415" @default.
- W4313331271 abstract "Near-field images of molecules provide information about their excited orbitals, giving rise to photonic and chemical functions. Such information is crucial to the elucidation of the full potential of molecules as components in functional materials and devices at the nanoscale. However, direct imaging inside single molecules with a complex structure in the near-field is still challenging because it requires in situ observation at a higher resolution than the molecular scale. Here, using a proven theoretical method that has demonstrated sub-nanoscale resolution based on photoinduced force microscopy (PiFM) experiment [ Nat. Commun. 12 , 3865 ( 2021 ) 10.1038/s41467-021-24136-2 ], we propose an approach to obtaining the near-field imaging with spatial patterns of electronic transitions of single molecules. We use an extended discrete dipole approximation method that incorporates microscopic nonlocal optical response of molecules and demonstrate that PiFM can visualize circular-dichroism signal patterns at sub-nanometer scale for both optically allowed and forbidden transitions. The result will open the possibility for the direct observation of complex spatial patterns of electronic transitions in a single molecule, providing insight into the optical function of single molecules and helping realize new functional materials and devices." @default.
- W4313331271 created "2023-01-06" @default.
- W4313331271 creator A5016735166 @default.
- W4313331271 creator A5016900470 @default.
- W4313331271 creator A5070687653 @default.
- W4313331271 creator A5071929627 @default.
- W4313331271 creator A5077394402 @default.
- W4313331271 date "2023-01-17" @default.
- W4313331271 modified "2023-10-14" @default.
- W4313331271 title "Near-field circular dichroism of single molecules" @default.
- W4313331271 cites W1963860368 @default.
- W4313331271 cites W1976722306 @default.
- W4313331271 cites W1986570163 @default.
- W4313331271 cites W1996851294 @default.
- W4313331271 cites W1998714697 @default.
- W4313331271 cites W1999173254 @default.
- W4313331271 cites W1999758799 @default.
- W4313331271 cites W2009482959 @default.
- W4313331271 cites W2010047724 @default.
- W4313331271 cites W2014678552 @default.
- W4313331271 cites W2022950330 @default.
- W4313331271 cites W2043007071 @default.
- W4313331271 cites W2070242211 @default.
- W4313331271 cites W2074325101 @default.
- W4313331271 cites W2115797520 @default.
- W4313331271 cites W2117567310 @default.
- W4313331271 cites W2170837376 @default.
- W4313331271 cites W2319891357 @default.
- W4313331271 cites W2323844726 @default.
- W4313331271 cites W2520235624 @default.
- W4313331271 cites W2524169139 @default.
- W4313331271 cites W2552717798 @default.
- W4313331271 cites W2560055168 @default.
- W4313331271 cites W2561531429 @default.
- W4313331271 cites W2599103843 @default.
- W4313331271 cites W2611172562 @default.
- W4313331271 cites W2694085773 @default.
- W4313331271 cites W2766482003 @default.
- W4313331271 cites W2777639606 @default.
- W4313331271 cites W2787663363 @default.
- W4313331271 cites W2789678565 @default.
- W4313331271 cites W2797885524 @default.
- W4313331271 cites W2885464240 @default.
- W4313331271 cites W2935271152 @default.
- W4313331271 cites W2952397553 @default.
- W4313331271 cites W2969986684 @default.
- W4313331271 cites W2983847778 @default.
- W4313331271 cites W3047800843 @default.
- W4313331271 cites W3089069763 @default.
- W4313331271 cites W3094201719 @default.
- W4313331271 cites W3174410274 @default.
- W4313331271 cites W3176166916 @default.
- W4313331271 cites W3190337842 @default.
- W4313331271 cites W4210745080 @default.
- W4313331271 cites W4296709418 @default.
- W4313331271 doi "https://doi.org/10.1364/oe.476011" @default.
- W4313331271 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36785335" @default.
- W4313331271 hasPublicationYear "2023" @default.
- W4313331271 type Work @default.
- W4313331271 citedByCount "1" @default.
- W4313331271 countsByYear W43133312712023 @default.
- W4313331271 crossrefType "journal-article" @default.
- W4313331271 hasAuthorship W4313331271A5016735166 @default.
- W4313331271 hasAuthorship W4313331271A5016900470 @default.
- W4313331271 hasAuthorship W4313331271A5070687653 @default.
- W4313331271 hasAuthorship W4313331271A5071929627 @default.
- W4313331271 hasAuthorship W4313331271A5077394402 @default.
- W4313331271 hasBestOaLocation W43133312711 @default.
- W4313331271 hasConcept C120665830 @default.
- W4313331271 hasConcept C121332964 @default.
- W4313331271 hasConcept C133571119 @default.
- W4313331271 hasConcept C138268822 @default.
- W4313331271 hasConcept C154945302 @default.
- W4313331271 hasConcept C171250308 @default.
- W4313331271 hasConcept C173523689 @default.
- W4313331271 hasConcept C185592680 @default.
- W4313331271 hasConcept C192562407 @default.
- W4313331271 hasConcept C202444582 @default.
- W4313331271 hasConcept C20788544 @default.
- W4313331271 hasConcept C21799368 @default.
- W4313331271 hasConcept C26771246 @default.
- W4313331271 hasConcept C32909587 @default.
- W4313331271 hasConcept C33923547 @default.
- W4313331271 hasConcept C41008148 @default.
- W4313331271 hasConcept C45206210 @default.
- W4313331271 hasConcept C62520636 @default.
- W4313331271 hasConcept C77017923 @default.
- W4313331271 hasConcept C8010536 @default.
- W4313331271 hasConcept C9652623 @default.
- W4313331271 hasConceptScore W4313331271C120665830 @default.
- W4313331271 hasConceptScore W4313331271C121332964 @default.
- W4313331271 hasConceptScore W4313331271C133571119 @default.
- W4313331271 hasConceptScore W4313331271C138268822 @default.
- W4313331271 hasConceptScore W4313331271C154945302 @default.
- W4313331271 hasConceptScore W4313331271C171250308 @default.
- W4313331271 hasConceptScore W4313331271C173523689 @default.
- W4313331271 hasConceptScore W4313331271C185592680 @default.
- W4313331271 hasConceptScore W4313331271C192562407 @default.