Matches in SemOpenAlex for { <https://semopenalex.org/work/W4313340147> ?p ?o ?g. }
- W4313340147 endingPage "1326" @default.
- W4313340147 startingPage "1319" @default.
- W4313340147 abstract "When high-energy radiation passes through aqueous material, low-energy electrons are produced which cause DNA damage. Electronic states of anionic nucleobases have been suggested as an entrance channel to capture the electron. However, identifying these electronic resonances have been restricted to gas-phase electron-nucleobase studies and offer limited insight into the resonances available within the aqueous environment of DNA. Here, resonance and detachment energies of the micro-hydrated uracil pyrimidine nucleobase anion are determined by two-dimensional photoelectron spectroscopy and are shown to extrapolate linearly with cluster size. This extrapolation allows the corresponding resonance and detachment energies to be determined for uracil in aqueous solution as well as the reorganization energy associated with electron capture. Two shape resonances are clearly identified that can capture low-energy electrons and subsequently form the radical anion by solvent stabilization and internal conversion to the ground electronic state. The resonances and their dynamics probed here are the nucleobase-centered doorway states for low-energy electron capture and damage in DNA." @default.
- W4313340147 created "2023-01-06" @default.
- W4313340147 creator A5007246543 @default.
- W4313340147 creator A5058363958 @default.
- W4313340147 creator A5059490660 @default.
- W4313340147 date "2022-12-30" @default.
- W4313340147 modified "2023-10-05" @default.
- W4313340147 title "Low-Energy Shape Resonances of a Nucleobase in Water" @default.
- W4313340147 cites W1952634231 @default.
- W4313340147 cites W1986264513 @default.
- W4313340147 cites W1989580075 @default.
- W4313340147 cites W1993340236 @default.
- W4313340147 cites W1993544440 @default.
- W4313340147 cites W1994416660 @default.
- W4313340147 cites W2001270915 @default.
- W4313340147 cites W2002224144 @default.
- W4313340147 cites W2003270528 @default.
- W4313340147 cites W2005749087 @default.
- W4313340147 cites W2006094627 @default.
- W4313340147 cites W2010792750 @default.
- W4313340147 cites W2020590034 @default.
- W4313340147 cites W2023528074 @default.
- W4313340147 cites W2025329625 @default.
- W4313340147 cites W2027826252 @default.
- W4313340147 cites W2033451476 @default.
- W4313340147 cites W2051461498 @default.
- W4313340147 cites W2062436875 @default.
- W4313340147 cites W2063201110 @default.
- W4313340147 cites W2066981219 @default.
- W4313340147 cites W2073176614 @default.
- W4313340147 cites W2079289918 @default.
- W4313340147 cites W2085370902 @default.
- W4313340147 cites W2087067311 @default.
- W4313340147 cites W2091237955 @default.
- W4313340147 cites W2101608919 @default.
- W4313340147 cites W2103970735 @default.
- W4313340147 cites W2106456081 @default.
- W4313340147 cites W2112434014 @default.
- W4313340147 cites W2132292065 @default.
- W4313340147 cites W2151248432 @default.
- W4313340147 cites W2166603911 @default.
- W4313340147 cites W2315301226 @default.
- W4313340147 cites W2316292712 @default.
- W4313340147 cites W2329299454 @default.
- W4313340147 cites W2515563452 @default.
- W4313340147 cites W2542177455 @default.
- W4313340147 cites W2584696766 @default.
- W4313340147 cites W2736542992 @default.
- W4313340147 cites W2742992791 @default.
- W4313340147 cites W2771249290 @default.
- W4313340147 cites W2783582260 @default.
- W4313340147 cites W2795469997 @default.
- W4313340147 cites W2801234511 @default.
- W4313340147 cites W2914857698 @default.
- W4313340147 cites W2950960607 @default.
- W4313340147 cites W2950969036 @default.
- W4313340147 cites W2973290003 @default.
- W4313340147 cites W3007660512 @default.
- W4313340147 cites W3021266098 @default.
- W4313340147 cites W3026952678 @default.
- W4313340147 cites W3115988671 @default.
- W4313340147 cites W3157916978 @default.
- W4313340147 cites W3183728106 @default.
- W4313340147 cites W3190761581 @default.
- W4313340147 cites W3191278063 @default.
- W4313340147 cites W4213340239 @default.
- W4313340147 cites W4224003060 @default.
- W4313340147 doi "https://doi.org/10.1021/jacs.2c11440" @default.
- W4313340147 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36584340" @default.
- W4313340147 hasPublicationYear "2022" @default.
- W4313340147 type Work @default.
- W4313340147 citedByCount "4" @default.
- W4313340147 countsByYear W43133401472023 @default.
- W4313340147 crossrefType "journal-article" @default.
- W4313340147 hasAuthorship W4313340147A5007246543 @default.
- W4313340147 hasAuthorship W4313340147A5058363958 @default.
- W4313340147 hasAuthorship W4313340147A5059490660 @default.
- W4313340147 hasBestOaLocation W43133401471 @default.
- W4313340147 hasConcept C105066094 @default.
- W4313340147 hasConcept C121332964 @default.
- W4313340147 hasConcept C139210041 @default.
- W4313340147 hasConcept C145148216 @default.
- W4313340147 hasConcept C147120987 @default.
- W4313340147 hasConcept C147789679 @default.
- W4313340147 hasConcept C159467904 @default.
- W4313340147 hasConcept C175708663 @default.
- W4313340147 hasConcept C178790620 @default.
- W4313340147 hasConcept C184651966 @default.
- W4313340147 hasConcept C184779094 @default.
- W4313340147 hasConcept C185592680 @default.
- W4313340147 hasConcept C187961010 @default.
- W4313340147 hasConcept C2779554091 @default.
- W4313340147 hasConcept C42296456 @default.
- W4313340147 hasConcept C46141821 @default.
- W4313340147 hasConcept C552990157 @default.
- W4313340147 hasConcept C55493867 @default.
- W4313340147 hasConcept C61234307 @default.
- W4313340147 hasConcept C62520636 @default.