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- W4313346265 abstract "Electrocatalysis of CO2 to CO is not only conducive to the artificial carbon cycle, but also green and efficient technology for producing chemicals. In consideration of the practical application, the novel strategy for large-scale preparation of catalyst has great potential to be developed. Herein, a facile one-step approach was developed for constructing a group of N-doping carbon-encapsulated metal catalysts ([email protected]C (M = Fe, Co, and Ni)) for CO2 electroreduction to CO. In addition, the impact of metal on catalytic performance was detailedly researched. Specifically, the [email protected]C catalyst achieves an excessive CO Faraday efficiency (FECO) (>90 %) on a broad achievable potential window of − 0.67 V to − 0.97 V vs RHE in the H-type cell. The optimal catalyst attains a FECO of 98 % at − 0.57 V vs RHE and an industrial-relevant current density of 430 mA cm−2 at − 1.07 V vs RHE in the flow cell. This work provides a facile way to fabricate catalyst on a large scale with preeminent performance for industrial CO2 electroreduction to CO." @default.
- W4313346265 created "2023-01-06" @default.
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- W4313346265 date "2023-03-01" @default.
- W4313346265 modified "2023-10-17" @default.
- W4313346265 title "Facile synthesis of N-doping carbon-encapsulated metal catalyst for CO2 electroreduction to CO" @default.
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- W4313346265 doi "https://doi.org/10.1016/j.apsusc.2022.156281" @default.
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