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- W4313357439 abstract "Abstract Despite the great progress of flexible perovskite solar cells (f‐PSCs), it still faces several challenges during the homogeneous fabrication of high‐quality perovskite thin films, and overcoming the insufficient exciton dissociation. To the ends, we rationally design the ferroelectric two‐dimensional (2D) perovskite based on pyridine heterocyclic ring as the organic interlayer. We uncover that incorporation of the ferroelectric 2D material into 3D perovskite induces an increased built‐in electric field (BEF), which enhances the exciton dissociation efficiency in the device. Moreover, the 2D seeds could assist the 3D crystallization by forming more homogeneous and highly‐oriented perovskite crystals. As a result, an impressive power conversion efficiency (PCE) over 23 % has been achieved by the f‐PSCs with outstanding ambient stability. Moreover, the piezo/ferroelectric 2D perovskite intrigues a decreased hole transport barriers at the ITO/perovskite interface under tensile stress, which opens new possibilities for developing highly‐efficient f‐PSCs." @default.
- W4313357439 created "2023-01-06" @default.
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- W4313357439 date "2023-01-18" @default.
- W4313357439 modified "2023-10-17" @default.
- W4313357439 title "Rational Design of Ferroelectric 2D Perovskite for Improving the Efficiency of Flexible Perovskite Solar Cells Over 23 %" @default.
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- W4313357439 doi "https://doi.org/10.1002/ange.202217526" @default.
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