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- W4313367817 abstract "The external oxidant-free exploitation of abundant alkane feedstocks as alkyl radical precursors remains a topic of high interest in synthetic communities. Here, we report a Ce-catalyzed electrophotoredox radical addition/cyclization cascade for the incorporation of unactivated alkanes to produce alkylated benzimidazo-fused isoquinolinones and other N-containing polycycles. Compared with previous works employing prefunctionalized alkyl radical precursors, this electrophotocatalytic protocol features high step-economy. The external oxidant-free conditions accompanied by the generation of H2 as the only byproduct further highlight the high redox- and atom-economy of this catalytic protocol." @default.
- W4313367817 created "2023-01-06" @default.
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- W4313367817 date "2023-01-01" @default.
- W4313367817 modified "2023-09-26" @default.
- W4313367817 title "Electrophotoredox/cerium-catalyzed unactivated alkanes activation for the sustainable synthesis of alkylated benzimidazo-fused isoquinolinones" @default.
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- W4313367817 doi "https://doi.org/10.1016/j.jcat.2022.12.033" @default.
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