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- W4313368319 endingPage "156180" @default.
- W4313368319 startingPage "156180" @default.
- W4313368319 abstract "Polymeric coatings are easy to be damaged by harsh environment condition, which causes cracks and loss of function. Inspired by the natural self-healing phenomenon, we successfully synthesized dual-functional cellulose nanocrystals/fluorinated polyacrylate containing coumarin derivatives by RAFT-assisted Pickering emulsion polymerization. The amphiphilic and photo-responsive copolymer, PDMAEMA-b-PGMA-b-P(HFBA-co-VBMC) was synthesized by RAFT process, followed by characterization using FT-IR, SEC, 1H NMR and UV–vis. The cellulose nanocrystals were modified by the copolymer, which were confirmed via XPS, UV–vis and so on. Besides, the droplet size of Pickering emulsion gradually increased and the creaming layer gradually decreased as the pH value increased. The TEM result showed that the modified cellulose nanocrystals were effectively anchored on the outside of latex particles. The size of the spherical-like latex particles increased and the stability of latex particles was worse with increasing pH value. Finally, the finished fabric had excellent water resistance due to the combination of micro- or nanoscale hierarchical structure and low surface energy. Moreover, the latex film exhibited excellent repeatability of self-healing ability. The fabric coating achieved the intrinsic and superficial dual-functional self-healing performance by the reversible [2 + 2] cycloaddition of coumarin groups. This strategy provides a powerful guide for preparing the high-performance waterborne fluorinated polyacrylate coating." @default.
- W4313368319 created "2023-01-06" @default.
- W4313368319 creator A5014068004 @default.
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- W4313368319 date "2023-03-01" @default.
- W4313368319 modified "2023-09-30" @default.
- W4313368319 title "Fabrication of dual-functional cellulose nanocrystals/fluorinated polyacrylate containing coumarin derivatives by RAFT-assisted Pickering emulsion polymerization for self-healing application" @default.
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- W4313368319 doi "https://doi.org/10.1016/j.apsusc.2022.156180" @default.
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