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- W4313377497 abstract "The practical implementation of Li metal has been severely obstructed by the uncontrolled dendritic Li growth and poor cycling efficiency. Herein, highly lithiophilic, ultrathin (∼60 nm) and conformal bismuth-oxygen-carbon layer-modified carbon fibers (CF@BOC) first prepared from the bismuth-based MOF membrane self-assembly were rationally adopted to stabilize Li metal. Highly efficient ultrasmall (∼1.8 nm) bismuth seeds and in-situ generated Li2O-enriched interphase can cooperatively enable the homogeneous Li nucleation/growth and extraordinarily high Li utilization efficiency. Consequently, the modified Li metal exhibits ultrahigh rate capability (10 mA cm−2) and ultralong lifespan stability (6900 cycles). Impressively, the Li|LiFePO4 full cell delivers an exceptional long-term cycling over 200 cycles under the rather harsh condition of low negative-to-positive-capacity (N/P) ratio (∼0.44) and electrolyte-to-capacity (E/C) ratio (5 g Ah−1). And the Li|LiCoO2 full cell also reveals a prolonged cycling performance even at the ultralow N/P ratio (∼0.26) with a remarkable energy density of 361.3 Wh kg−1. Furthermore, the pouch cell with a high loading cathode (3.6 mAh cm−2) still demonstrates prolonged cycling lifespan under the practical condition of extremely limited Li metal and lean electrolyte. This work enlightens a significant stride toward highly stable Li metal anode for practicability." @default.
- W4313377497 created "2023-01-06" @default.
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- W4313377497 date "2023-01-01" @default.
- W4313377497 modified "2023-10-14" @default.
- W4313377497 title "Cooperative stabilization by highly efficient nanoseeds and reinforced interphase toward practical Li metal batteries" @default.
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- W4313377497 doi "https://doi.org/10.1016/j.ensm.2022.12.017" @default.
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