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- W4313377967 abstract "Abstract Developing new materials for anhydrous proton conduction under high‐temperature conditions is significant and challenging. Herein, we create a series of highly crystalline covalent organic frameworks (COFs) via a pore engineering approach. We simultaneously engineer the pore geometry (generating concave dodecagonal nanopores) and pore surface (installing multiple functional groups such as −C=N−, −OH, −N=N− and −CF 3 ) to improve the utilization efficiency and host–guest interaction of proton carriers, hence benefiting the enhancement of anhydrous proton conduction. Upon loading with H 3 PO 4 , COFs can realize a proton conductivity of 2.33×10 −2 S cm −1 under anhydrous conditions, among the highest values of all COF materials. These materials demonstrate good stability and maintain high proton conductivity over a wide temperature range (80–160 °C). This work paves a new way for designing COFs for anhydrous proton conduction applications, which shows great potential as high‐temperature proton exchange membranes." @default.
- W4313377967 created "2023-01-06" @default.
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- W4313377967 date "2022-12-29" @default.
- W4313377967 modified "2023-10-17" @default.
- W4313377967 title "Pore Geometry and Surface Engineering of Covalent Organic Frameworks for Anhydrous Proton Conduction" @default.
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- W4313377967 doi "https://doi.org/10.1002/ange.202217240" @default.
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