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• W4313405412 abstract "The cathode materials work as the host framework for both Li+ diffusion and electron transport in Li-ion batteries. The Li+ diffusion property is always the research focus, while the electron transport property is less studied. Herein, we propose a unique strategy to elevate the rate performance through promoting the surface electric conductivity. Specifically, a disordered rock-salt phase was coherently constructed at the surface of LiCoO2 , promoting the surface electric conductivity by over one magnitude. It increased the effective voltage (Veff ) imposed in the bulk, thus driving more Li+ extraction/insertion and making LiCoO2 exhibit superior rate capability (154 mAh g-1 at 10 C), and excellent cycling performance (93 % after 1000 cycles at 10 C). The universality of this strategy was confirmed by another surface design and a simulation. Our findings provide a new angle for developing high-rate cathode materials by tuning the surface electron transport property." @default.
• W4313405412 created "2023-01-06" @default.
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• W4313405412 date "2023-01-24" @default.
• W4313405412 modified "2023-10-14" @default.
• W4313405412 title "Promoting Surface Electric Conductivity for High‐Rate LiCoO ₂" @default.
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• W4313405412 doi "https://doi.org/10.1002/anie.202218595" @default.
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• W4313405412 hasPublicationYear "2023" @default.
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