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• W4313419746 endingPage "232538" @default.
• W4313419746 startingPage "232538" @default.
• W4313419746 abstract "Lead-acid battery technology continues to form a critical part of the global electrochemical energy storage market. Part of the reason for the lead-acid battery's success is due to its well understood electrochemistry. However, over recent years it has become clear that a poor understanding of inherent heterogeneity in chemical changes that happen during the charge and discharge cycles of these batteries is limiting innovation. In this paper we show that high-energy X-rays can be used to better understand how the chemistry within these systems is localised spatially, and how it affects battery performance. Used commercial lead-acid battery electrodes were sampled then imaged before and after the Pb K-edge (88 keV). In these electrodes, multiple features associated with battery failure were clearly observed throughout each electrode. A custom-made lead-acid battery was also imaged in-operando. Inhomogeneous utilization of the negative electrode arising from charge-transport effects could be clearly observed in the electrode face. These results show that high-energy X-ray imaging could be a powerful tool to better understand the relationship between the spatial and electrochemical dimensions in lead-acid batteries." @default.
• W4313419746 created "2023-01-06" @default.
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• W4313419746 date "2023-02-01" @default.
• W4313419746 modified "2023-09-25" @default.
• W4313419746 title "High energy X-ray imaging of heterogeneity in charged and discharged lead-acid battery electrodes" @default.
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• W4313419746 doi "https://doi.org/10.1016/j.jpowsour.2022.232538" @default.
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