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• W4313442935 abstract "Selective electrodialysis (SED) method has been proved to be effective in the process of the removal of mental ions from the ionic liquid (IL) aqueous solution in our previous work. However, the membrane fouling and cleaning strategy have not yet been investigated in IL recovery process, which are essential issues concerning the membrane life and overall cost. Therefore, various operating parameters, i.e. operation time, metal ion concentration, IL concentration, pH and temperature were systematically investigated to reveal the formation of membrane fouling in this work. Then, basing on the analysis results of fouling formation, the ion exchange capacity (IEC), contact angle, resistance, XPS were further adopted to reveal the fouling mechanism. These results showed that the variation of physicochemical properties of membranes with the formation of membrane fouling, and the [Emim]+ cation combined with the fixed groups in MSCM through physical/chemical formation. The EIS further demonstrated that the ion migration path changed as for the formation of [Emim]+, Mg2+, Ca2+ fouling layer. Finally, inspired by this mechanism, a specific cleaning strategy with the order of H2O, 0.1 M HCl, and 0.1 M NaCl was proposed, and the membranes exhibited the steady separation performance and physicochemical properties within 6-times recycle." @default.
• W4313442935 created "2023-01-06" @default.
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• W4313442935 date "2023-02-01" @default.
• W4313442935 modified "2023-10-14" @default.
• W4313442935 title "Insight into membrane fouling mechanism and cleaning strategy during selective electrodialysis for metal ions removal from ionic liquid aqueous solutions" @default.
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• W4313442935 doi "https://doi.org/10.1016/j.jece.2022.109246" @default.
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