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- W4313443570 abstract "The development of highly efficient and reliable adsorbent towards radiactive 99TcO4− is of great significance. Here, a covalent polymeric network (Py-CPN) based on pyridinium was rationally designed and synthesized through nucleophilic substitution reaction between 3D building unit tetrakis(4-(bromomethyl) phenyl) methane (TBPM) and 1,3,6,8-tetra(pyridin-4-yl) pyrene (TPyPy). Due to the rigidity and shape-persistence of tetrahedral unit of TBPM, which benefited rapid ion transportation across the polymeric network, Py-CPN provided high adsorption capacity and fast kinetics towards ReO4− removal. Owing to the introduction of highly hydrophobic and largely conjugated monomer TPyPy, excellent selectivity towards various coexisting anions was achieved. Moreover, the sorption ability of Py-CPN remained stable over a wide range of pH values, including 3 M HNO3 solution and simulated Hanford LAW off-gas recycle wastes. Py-CPN also exhibited excellent recyclability for at least four cycles. Overall, this work provided a new strategy for constructing high-performance polymeric materials for sustainable development of environment protection." @default.
- W4313443570 created "2023-01-06" @default.
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- W4313443570 date "2023-03-01" @default.
- W4313443570 modified "2023-10-09" @default.
- W4313443570 title "Rationally designed pyridinium cationic polymeric network for effective TcO4−/ReO4− remediation" @default.
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- W4313443570 doi "https://doi.org/10.1016/j.ces.2022.118403" @default.
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