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- W4313443676 abstract "Limited transport and migration of photoinduced charges in polymeric carbon nitride (g-C3N4) within the planar layers remain a great challenge for achieving favorable photocatalysis. Herein, phosphorus-doped carbon quantum dots (PCDots) implanted intra-layer carbon nitride nanosheet (PCDots-C3N4) photocatalyst with phosphorus-nitrogen (P–N) bridging was prepared. The 13C and 31P of nuclear magnetic resonance, X-ray photoelectron spectroscopy, and density functional theory calculations confirmed the formation of a P–N bridge. Additionally, implanting PCDots enlarged the π-π conjugated electronic structure and modulated the plane structure of g-C3N4. The atomic-level connection by the P–N bridge dramatically extended the delocalization effect and facilitated the intramolecular charge transfer. PCDots-C3N4 demonstrated efficient photodegradation of tetracycline hydrochloride (TC) and bisphenol A (BPA) than both g-C3N4 and CDots-C3N4, reaching 76% and 100%, respectively. The possible degradation pathways of TC and BPA were also discussed. This work provides an efficient strategy for rapid electron transfer to form a new paradigm for wastewater remediation." @default.
- W4313443676 created "2023-01-06" @default.
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- W4313443676 date "2023-02-01" @default.
- W4313443676 modified "2023-10-16" @default.
- W4313443676 title "Unraveling the phosphorus-nitrogen bridge in carbon quantum dots/carbon nitride for efficient photodegradation of organic contaminants" @default.
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- W4313443676 doi "https://doi.org/10.1016/j.carbon.2022.12.063" @default.
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