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- W4313451746 abstract "Success in the development of aqueous batteries hinges on strict design principles for the aqueous electrolyte: utilize the high ionic conductivity but limit the redox activity of water. Here we develop a new type of electrolyte, a “water-in-ionic liquid” electrolyte, where the water molecule is sealed in a water trap composed of ions by short-range intermolecular interactions. In this way, the water molecule is protected by the surrounding anion-abundant framework and simultaneously plays its lubricant role for ionic conduction, realizing a high stability together with a high ionic conductivity (1.18 × 10–2 S cm–1) of the electrolyte. This water-confined motif promotes the formation of an explicit interphase (SEI) on a Zn metal anode, which is clearly observed for the first time and contributes to a substantially reversible Zn electrochemistry. Notably, due to the intermolecular constraint, the volatilization of this electrolyte is alleviated, which is helpful for batteries with an open system. As a proof of concept, we demonstrate zinc–air batteries (ZABs) with superior longevity compared to those using typical aqueous electrolyte under lean-electrolyte conditions (300 h vs 72 h, respectively)." @default.
- W4313451746 created "2023-01-06" @default.
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- W4313451746 date "2022-12-20" @default.
- W4313451746 modified "2023-10-16" @default.
- W4313451746 title "A Novel “Water-in-Ionic Liquid” Electrolyte for Zn Metal Batteries" @default.
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- W4313451746 doi "https://doi.org/10.1021/acsenergylett.2c02520" @default.
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