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• W4313453404 abstract "Ammonium ions (NH4+ ), as non-metallic charge carriers, are attracting attention in aqueous batteries due to its low molar mass, element sufficiency, and non-toxicity. However, the host materials for NH4+ storage are still limited. Herein, an oxygen defects-rich manganese oxide (MnO2-x ) for NH4+ storage are reported. The oxygen defects can endow the MnO2-x sample with improved electric conductivity and low interface activation energy. The electrochemical reaction mechanism is also verified by using ex situ X-ray photoelectron spectroscopy (XPS) and fourier transform infrared spectroscopy (FT-IR), demonstrating the insertion and extraction of NH4+ in the MnO2-x by formation/breaking of a hydrogen bond. As a result, MnO2-x delivers a high capacity of 109.9 mAh g-1 at the current density of 0.5 A g-1 and retention of 24 mAh g-1 after 1000 cycles at the current density of 4 A g-1 , outperforming the pristine MnO2 sample." @default.
• W4313453404 created "2023-01-06" @default.
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• W4313453404 date "2023-01-02" @default.
• W4313453404 modified "2023-10-17" @default.
• W4313453404 title "Valence Engineering Enhancing NH₄⁺ Storage Capacity of Manganese Oxides" @default.
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• W4313453404 doi "https://doi.org/10.1002/smll.202206727" @default.
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