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- W4313454265 abstract "The site-selective functionalization of unactivated allylic C-H bonds via direct deprotonation using KTMP is described. The conversion of amorphadiene to artemisinic alcohol via a simple, highly regioselective deprotonation over 4 other possible allylic sites is shown with further extrapolation to the first large-scale telescoped chemical synthesis of artemisinic acid from amorphadiene. Finally, application of the method for the successful site-selective functionalization of unactivated allylic C-H bonds in other terpene-based natural products is also highlighted." @default.
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- W4313454265 date "2023-01-02" @default.
- W4313454265 modified "2023-10-18" @default.
- W4313454265 title "Site-Selective Functionalization of Unactivated Allylic C–H Bonds via Direct Deprotonation with KTMP: Application to the Formal Total Synthesis of (+)-Artemisinin from Amorphadiene" @default.
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- W4313454265 doi "https://doi.org/10.1021/acs.orglett.2c04145" @default.
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