Matches in SemOpenAlex for { <https://semopenalex.org/work/W4313455005> ?p ?o ?g. }
- W4313455005 abstract "Albeit considerable attention to the fast-developing organic thermoelectric (OTE) materials due to their flexibility and non-toxic features, it is still challenging to design an OTE polymer with superior thermoelectric properties. In this work, two isomorphic donor-acceptor (D-A) conjugated polymers are studied as the semiconductor in OTE devices, revealing for the first time the internal mechanism of regioregularity on thermoelectric performances in D-A type polymers. A higher molecular structure regularity can lead to higher crystalline order and mobility, higher doping efficiency, order of energy state, and thermoelectric (TE) performance. As a result, the regioregular P2F exhibits a maximum power factor (PF) of up to 113.27 µW m-1 K-2 , more than three times that of the regiorandom PRF (35.35 µW m-1 K-2 ). However, the regular backbone also implies lower miscibility with a dopant, negatively affecting TE performance. Therefore, the trade-off between doping efficiency and miscibility plays a vital role in OTE materials, and this work sheds light on the molecular design strategy of OTE polymers with state-of-the-art performances." @default.
- W4313455005 created "2023-01-06" @default.
- W4313455005 creator A5006688405 @default.
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- W4313455005 creator A5088834856 @default.
- W4313455005 date "2023-01-02" @default.
- W4313455005 modified "2023-10-17" @default.
- W4313455005 title "Revealing the Enhanced Thermoelectric Properties of Controllably Doped Donor‐Acceptor Copolymer: The Impact of Regioregularity" @default.
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