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- W4313458841 abstract "The present study reports an asymmetric NHC-catalyzed formal [4 + 2] cycloaddition of heterocyclic alkenes containing a polarized double bond with an azolium-dienolate intermediate generated from α-bromo-α,β-unsaturated aldehydes without external oxidation of the Breslow intermediate. Heterocyclic cyclohexenones were produced in good isolated yields (typically about 90%) with good stereochemical outcomes (in most cases, dr > 20/1, and ee = 70-99%). The synthetic utility of the protocol was exemplified by the scope of heterocyclic alkenes." @default.
- W4313458841 created "2023-01-06" @default.
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- W4313458841 date "2023-01-03" @default.
- W4313458841 modified "2023-10-03" @default.
- W4313458841 title "Stereoselective <i>N</i>-Heterocyclic-Carbene-Catalyzed Formal [4 + 2] Cycloaddition: Access to Chiral Heterocyclic Cyclohexenones" @default.
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- W4313458841 doi "https://doi.org/10.1021/acs.orglett.2c04021" @default.
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