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- W4313481356 abstract "Tailoring the lithium-ion solvation structure of ether-based electrolyte to accelerate charge transfer is of significance in low-temperature lithium batteries but remains largely unexplored. Herein, we propose a strategy based on carbonates mediating the anion coordination to realize cold-resistant electrolyte with superior kinetics and improved anodic stability. The combination of computational and experimental methods reveals that decreasing anions in the Li+-solvation structure reduces the desolvation energy of Li+ and enhances low-temperature performance. A formulated electrolyte composed of 0.5 M lithium tetrafluoroborate in hybrid solvent of tetrahydrofuran and trifluoropropylene carbonate features a high ionic conductivity of 0.45 mS cm−1 at − 90 °C and an ultra-low freezing point of − 133 °C. Furthermore, in such electrolyte, the LiNi0.8Co0.1Mn0.1O2 cathode can be reversibly cycled at low temperature of − 40 °C and delivers a considerable specific capacity of 108.5 mAh/g at − 90 °C." @default.
- W4313481356 created "2023-01-06" @default.
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- W4313481356 date "2023-02-01" @default.
- W4313481356 modified "2023-10-15" @default.
- W4313481356 title "Non-concentrated electrolyte with weak anion coordination enables low Li-ion desolvation energy for low-temperature lithium batteries" @default.
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- W4313481356 doi "https://doi.org/10.1016/j.cej.2023.141273" @default.
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