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• W4313487997 abstract "Herein, we fabricated a π-π stacking hybrid photocatalyst by combining two two-dimensional (2D) materials: g-C3 N4 and a Cu-porphyrin metal-organic framework (MOF). After an aerobic photocatalytic pretreatment, this hybrid catalyst exhibited an unprecedented ability to photocatalytically reduce CO2 to CO and CH4 under the typical level (20 %) of O2 in the air. Intriguingly, the presence of O2 did not suppress CO2 reduction; instead, a fivefold increase compared with that in the absence of O2 was observed. Structural analysis indicated that during aerobic pretreatment, the Cu node in the 2D-MOF moiety was hydroxylated by the hydroxyl generated from the reduction of O2 . Then the formed hydroxylated Cu node maintained its structure during aerobic CO2 reduction, whereas it underwent structural alteration and was reductively devitalized in the absence of O2 . Theoretical calculations further demonstrated that CO2 reduction, instead of O2 reduction, occurred preferentially on the hydroxylated Cu node." @default.
• W4313487997 created "2023-01-06" @default.
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• W4313487997 date "2023-01-25" @default.
• W4313487997 modified "2023-10-17" @default.
• W4313487997 title "Facilitated Photocatalytic CO₂ Reduction in Aerobic Environment on a Copper‐Porphyrin Metal–Organic Framework" @default.
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• W4313487997 doi "https://doi.org/10.1002/anie.202216717" @default.
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