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• W4313488504 abstract "The first diastereoselective synthesis of trisubstituted cubanes was achieved using a chiral auxiliary. To establish chirality within the cubane skeleton, at least three substituents must be introduced at the appropriate positions. Ready conversion of cubane carboxylic acid to a chiral amide followed by sequential ortho-selective deprotonations and electrophilic trapping afforded the corresponding 1,2,3-trisubstituted cubanes with high diastereoselectivity. This route opens new possibilities for the preparation of enantio-enriched cubanes." @default.
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• W4313488504 date "2023-01-03" @default.
• W4313488504 modified "2023-10-05" @default.
• W4313488504 title "Chiral Auxiliary-Directed Site-Selective Deprotonation of the Cubane Skeleton" @default.
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• W4313488504 doi "https://doi.org/10.1021/acs.orglett.2c03659" @default.
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