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• W4313506239 endingPage "140905" @default.
• W4313506239 startingPage "140905" @default.
• W4313506239 abstract "Nowadays, metal–organic framework-derived (MOF-D) materials are auspicious in various research areas due to their beneficial traits of diverse structural features, large surface area, and high porous nature. Herein, we report the MOF-D nickel–cobalt terephthalate hydroxides (Ni-Co THs) via a one-pot solvothermal approach without further annealing. Direct growth of active materials on conductive substrates (e.g., nickel foam (NF)) can potentially eliminate the use of sluggish and non-conductive binders, leading to enhanced redox chemistry with commercial-level mass loading (8–10 mg cm−2). All the binder-free MOF-D Ni-Co TH electrodes demonstrated excellent areal capacities at the same current density of 3 mA cm−2. Among them, the Ni-Co TH-160/9h electrode delivered a superior areal capacity/specific capacity of 2087 µAh cm−2/200.68 mAh g−1 at 3 mA cm−2, together with outstanding cycling retention of 100 % after 20,000 charge–discharge cycles. The achieved ultrahigh performance is ascribed to the synergistic properties of Ni-Co THs, three-dimensional porous NF, and morphological structures. Utilizing the charge storage performance of the Ni-Co TH-160/9h electrode, an electrochemical cell (ECC) was assembled. The as-assembled ECC delivered good areal capacity (1678.6 µAh cm−2), energy density (1.3 mWh cm−2), and power density (48.6 mW cm−2) with outstanding cycling performance (35,000 cycles (99.9 %)). Also, the ECC verified its energy storage properties by powering various portable electronic appliances." @default.
• W4313506239 created "2023-01-06" @default.
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• W4313506239 date "2023-01-01" @default.
• W4313506239 modified "2023-10-16" @default.
• W4313506239 title "Design of high-mass loading metal–organic framework-based electrode materials with excellent redox activity for long-lasting electrochemical energy storage applications" @default.
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• W4313506239 doi "https://doi.org/10.1016/j.cej.2022.140905" @default.
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