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- W4313528075 abstract "In this work, we numerically investigate the impact of two-dimensional solute gradients on the distribution of colloidal particles, i.e., colloidal banding, induced via diffusiophoresis. The solute gradients are generated by spatially arranged sources and sinks that emit/absorb a time-dependent solute flux. First we study a dipole system, i.e., one source and one sink, and discover that interdipole diffusion and flux decay timescales dictate colloidal banding. At timescales shorter than the interdipole diffusion timescale, we observe a rapid enhancement in particle enrichment around the source due to repulsion from the sink. However, at timescales longer than the interdipole diffusion timescale, the source and sink screen each other, leading to a slower enhancement. If the solute flux decays at the timescale of interdipole diffusion, an optimal separation distance is obtained such that particle enrichment is maximized. We find that the partition coefficient between solute inside the source and the bulk strongly impacts the optimal separation distance. Surprisingly, the diffusivity ratio between solute in the source and bulk has a much weaker impact on the optimal dipole separation distance. We also examine an octupole configuration, i.e., four sinks and four sources, arranged in a circle, and demonstrate that the geometric arrangement that maximizes enrichment depends on the radius of the circle. If the radius of the circle is small, it is preferred to have sources and sinks arranged in an alternating fashion. However, if the radius of the circle is large, a consecutive arrangement of sources and sinks is optimal. Our numerical framework introduces a novel method for spatially and temporally designing the banded structure of colloidal particles in two dimensions using diffusiophoresis and opens up new avenues in a field that has primarily focused on one-dimensional solute gradients." @default.
- W4313528075 created "2023-01-06" @default.
- W4313528075 creator A5014338118 @default.
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- W4313528075 creator A5081180707 @default.
- W4313528075 date "2023-01-01" @default.
- W4313528075 modified "2023-09-27" @default.
- W4313528075 title "Two-dimensional diffusiophoretic colloidal banding: optimizing the spatial and temporal design of solute sinks and sources" @default.
- W4313528075 cites W1969613862 @default.
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- W4313528075 cites W1988818744 @default.
- W4313528075 cites W1998513022 @default.
- W4313528075 cites W2001962804 @default.
- W4313528075 cites W2024851651 @default.
- W4313528075 cites W2033949377 @default.
- W4313528075 cites W2060727516 @default.
- W4313528075 cites W2062288737 @default.
- W4313528075 cites W2063098299 @default.
- W4313528075 cites W2081486859 @default.
- W4313528075 cites W2083657299 @default.
- W4313528075 cites W2086783605 @default.
- W4313528075 cites W2088115535 @default.
- W4313528075 cites W2119398509 @default.
- W4313528075 cites W2123790526 @default.
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- W4313528075 cites W2567041579 @default.
- W4313528075 cites W2568687711 @default.
- W4313528075 cites W2611161933 @default.
- W4313528075 cites W2624260436 @default.
- W4313528075 cites W2725480271 @default.
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- W4313528075 doi "https://doi.org/10.1039/d2sm01549h" @default.
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- W4313528075 hasPublicationYear "2023" @default.
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