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- W4313531263 abstract "Aiming at enhancing the detection of phenolic contaminants in high-temperature environments, we developed a thermoregulatory electrochemical biosensor based on the tyrosinase-immobilized electroactive phase-change microcapsules. The microcapsules were fabricated by engulfing n-eicosane as a phase-change material core in a TiO2 shell, followed by depositing with an electroactive hybrid layer comprising the polypyrrole matrix and tyrosinase-immobilized Fe3O4 nanoparticles. The resultant microcapsules show a well-defined core–shell microstructure and a regular spherical morphology, together with the desired chemical compositions and structures. Acting as a biosensing electrode material, the microcapsules exhibit a high latent heat capacity of around 150 J/g to implement microenvironmental temperature regulation for the biosensor through reversible phase transitions of their n-eicosane core. This enables the developed biosensor to obtain a higher enzyme activity and more sensitive biosensing performance at high assay temperatures when compared to conventional tyrosinase biosensors, resulting in a high sensitivity of 0.102 (µA·L)/µmol and a lower detection limit of 3.409 µmol/L for catechol detection. Based on a unique integration of phase-change microcapsules and immobilized tyrosinase in the working electrode, the electrochemical biosensor developed in this study has found a practical application for high-sensitive reorganization and high-accurate determination of phenolic contaminants in industrial wastewaters over a wide working temperature range." @default.
- W4313531263 created "2023-01-06" @default.
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- W4313531263 date "2023-04-01" @default.
- W4313531263 modified "2023-10-15" @default.
- W4313531263 title "Electrochemical biosensor based on tyrosinase-immobilized phase-change microcapsules for ultrasensitive detection of phenolic contaminants under in situ thermal management" @default.
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- W4313531263 doi "https://doi.org/10.1016/j.jiec.2022.12.042" @default.
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