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• W4313532385 abstract "Abstract The MOF Ni(bdc)(ted) 0.5 was selected as the hydrogen isotope separation material in this paper and the separation mechanism of this material was investigated by molecular simulation. Theoretical calculations proved that Ni(bdc)(ted) 0.5 had chemical affinity quantum sieving (CAQS) effect and kinetic quantum sieving (KQS) effect. Because the adsorption capacity of D 2 in Ni(bdc)(ted) 0.5 was larger than H 2 and the diffusion rate was smaller than H 2 at 77 K, Ni(bdc)(ted) 0.5 could realize the separation of hydrogen and deuterium in gas chromatography. Ni(bdc)(ted) 0.5 @γ‐Al 2 O 3 composite was prepared by liquid phase epitaxy method as gas chromatographic packings (column type: 0.6 m×2.0 mm I.D.) to investigate the separation performance of H 2 /D 2 at 77 K. Under the optimal chromatographic conditions, the retention time of H 2 and D 2 were 1.95 and 3.48 min respectively and the resolution ( R ) was 2.12, indicating that the separation of H 2 and D 2 could be realized efficiently and quickly by using Ni(bdc)(ted) 0.5 @γ‐Al 2 O 3 ." @default.
• W4313532385 created "2023-01-06" @default.
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• W4313532385 date "2023-01-03" @default.
• W4313532385 modified "2023-10-12" @default.
• W4313532385 title "Quantum Sieving Effects of Ni(bdc)(ted)_0.5 and Effective Separation Performance of Ni(bdc)(ted)_0.5@γ‐Al₂O₃ for H₂/D₂" @default.
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• W4313532385 doi "https://doi.org/10.1002/slct.202204150" @default.
• W4313532385 hasPublicationYear "2023" @default.
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