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- W4313551738 abstract "Abstract Decreasing the catalytic loading and complexity of electrocatalysts for the reduction of CO 2 is a critical necessity towards globally generating carbon-negative synthons. This effort therefore calls for the development of not only more active catalysts per employed g but also for more financially sound ones. Notably, molecular electrocatalysts allow for tuning the electronic and geometric environment around single-atom catalytic centers. Nevertheless, synthetic complexity, cost and electrochemical instability still hamper their large-scale implementation. With industrial application in mind, we herein present a holistic design approach starting from different Ag(I) N,N´ -bis(arylimino)acenaphtene complexes to sophisticated architectures of electrolyzer components. Performed in industrially applicable cells at 60°C, this approach allows us to reach catalytic activity for CO formation close to 1 A cm -2 , while achieving the highest mass activity reported for CO at 100.000 A gA g -1 , accompanied by cost decreases up to a factor of 80 against the current heterogeneous standards. This study thus represents an unprecedented example to show the applicability of homogenous catalysts under industrially relevant conditions." @default.
- W4313551738 created "2023-01-06" @default.
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- W4313551738 date "2023-01-06" @default.
- W4313551738 modified "2023-10-16" @default.
- W4313551738 title "Ultra-low Ag Loadings for CO2 Reduction via Tailored Molecular Electrocatalysts" @default.
- W4313551738 doi "https://doi.org/10.21203/rs.3.rs-2353282/v1" @default.
- W4313551738 hasPublicationYear "2023" @default.
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