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• W4313552023 endingPage "3688" @default.
• W4313552023 startingPage "3680" @default.
• W4313552023 abstract "Electronic waste is a growing challenge which needs to be addressed through the integration of high-performance sustainable materials. Green dielectric polymers such as poly(vinyl alcohol) (PVA) have favorable electrical properties but are challenging to integrate into thin film electronics due to their physical properties. For example, PVA suffers from poor film formation and is hygroscopic. Bilayer dielectrics with interfacial cross-linking can enable the use of high-performance PVA with favorable surface chemistry by using a hydrophobic poly(caprolactone) (PCL) layer. In this study, we developed a benzodioxinone-terminated PCL layer, which can be UV cross-linked to the hydroxy groups of the PVA dielectric. This air-stable UV-cross-linking PCL dielectric was able to effectively cross-link with PVA, leading to high-performance capacitors and single-walled carbon nanotube-based thin film transistors. This UV cross-linking PCL dielectric led to significant improvements in shelf-life, ease of processing, and similar device performance compared to our previously reported thermally cross-linking PCL layer. The UV cross-linking at the interface between these bilayers can allow for the integration of high-speed roll-to-roll processing, which enables low-cost, sustainable, and high-performance electronics." @default.
• W4313552023 created "2023-01-06" @default.
• W4313552023 creator A5029544868 @default.
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• W4313552023 date "2023-01-05" @default.
• W4313552023 modified "2023-10-02" @default.
• W4313552023 title "Interfacial Ultraviolet Cross-Linking of Green Bilayer Dielectrics" @default.
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• W4313552023 doi "https://doi.org/10.1021/acsami.2c21412" @default.
• W4313552023 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36603855" @default.
• W4313552023 hasPublicationYear "2023" @default.
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