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- W4313554674 abstract "Single-particle spectroelectrochemistry provides optical insight into understanding physical and chemical changes occurring on the nanoscale. While changes in dark-field scattering during electrochemical charging are well understood, changes to the photoluminescence of plasmonic nanoparticles under similar conditions are less studied. Here, we use correlated single-particle photoluminescence and dark-field scattering to compare their plasmon modulation at applied potentials. We find that changes in the emission of a single gold nanorod during charge density tuning of intraband photoluminescence can be attributed to changes in the Purcell factor and absorption cross section. Finally, modulation of interband photoluminescence provides an additional constructive observable, giving promise for establishing dual channel sensing in spectroelectrochemical measurements." @default.
- W4313554674 created "2023-01-06" @default.
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- W4313554674 date "2023-01-05" @default.
- W4313554674 modified "2023-09-27" @default.
- W4313554674 title "Single-Particle Photoluminescence and Dark-Field Scattering during Charge Density Tuning" @default.
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- W4313554674 doi "https://doi.org/10.1021/acs.jpclett.2c03566" @default.
- W4313554674 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36603176" @default.
- W4313554674 hasPublicationYear "2023" @default.
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