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• W4313558881 abstract "Abstract We herein report two asymmetric germanate crystals, KNbGe 3 O 9 and K 3 Nb 3 Ge 2 O 13 , with different structures and optical properties derived from divergent polymerized forms of GeO 4 and NbO 6 groups. Remarkably, K 3 Nb 3 Ge 2 O 13 achieved a rare combination of the strongest second harmonic generation (SHG) response of 17.5×KDP @ 1064 nm and the largest birefringence of 0.196 @ 546 nm in germanates. It features unique [Nb 3 O 12 ] ∞ tubular chains constructed by circular Nb 3 O 15 tripolymers. Theoretical calculations reveal that the d ‐ p interactions in the Nb 3 O 15 group are responsible for outstanding optical properties. This work emphasizes the significance of the polymerizable functional units in obtaining high‐performance nonlinear optical (NLO) crystals." @default.
• W4313558881 created "2023-01-06" @default.
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• W4313558881 date "2023-01-24" @default.
• W4313558881 modified "2023-09-26" @default.
• W4313558881 title "Intense <i>d‐p</i> Hybridization in Nb₃O₁₅ Tripolymer Induced the Largest Second Harmonic Generation Response and Birefringence in Germanates" @default.
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• W4313558881 doi "https://doi.org/10.1002/ange.202217039" @default.
• W4313558881 hasPublicationYear "2023" @default.
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