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- W4313561334 abstract "The synthesis of zeolites from natural aluminosilicate minerals is environmentally sustainable. However, the preparation of nano-ZSM-5 zeolite single crystals via the facile “silica–alumina homologation” of natural clay remains challenging. This paper highlights a novel strategy for the synthesis of defect-free, highly crystalline nano-H-ZSM-5 with a uniform morphology through the kinetically controlled in situ reconstruction of the topology of natural clay within a solid-state-like system. Crystal nucleation and growth were decoupled by aging to control the crystal size. The “homogeneous silica–alumina” property of natural clay was found to be directly inherited by nano-H-ZSM-5 to provide uniformly distributed acidic sites for catalysis. This was demonstrated by methanol-to-propylene conversion, wherein the performance of the obtained crystals was superior to that of commercial ZSM-5. This strategy promotes the development of natural silica–aluminate clay resources and allows the scalable production of high-quality nano-H-ZSM-5 single crystals for heterogeneous catalysis." @default.
- W4313561334 created "2023-01-06" @default.
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- W4313561334 date "2023-02-01" @default.
- W4313561334 modified "2023-09-29" @default.
- W4313561334 title "Green synthesis of nano-H-ZSM-5 zeolite single-crystal aggregates via an in situ reconstruction of the topology of natural clay" @default.
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- W4313561334 doi "https://doi.org/10.1016/j.micromeso.2023.112441" @default.
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