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- W4313591983 abstract "Abstract Motivated by the discovery of superconductivity in KTaO 3 -based heterostructures, we study a pairing mechanism based on spin-orbit assisted coupling between the conduction electrons and the ferroelectric (FE) modes present in the material. We use ab initio frozen-phonon computations to show a linear-in-momentum Rashba-like coupling with a strong angular dependence in momentum for the lower <?CDATA $j = 3/2$?> <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML overflow=scroll> <mml:mi>j</mml:mi> <mml:mo>=</mml:mo> <mml:mn>3</mml:mn> <mml:mrow> <mml:mo>/</mml:mo> </mml:mrow> <mml:mn>2</mml:mn> </mml:math> manifold, deviating from the conventional isotropic Rashba model. This implies the Rashba-like interaction with the polar modes has substantial L = 3 cubic harmonic corrections, which we quantify for each electronic band. The strong anisotropy of the Rashba interaction is captured by a microscopic toy model for the <?CDATA $t_{2g}$?> <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML overflow=scroll> <mml:msub> <mml:mi>t</mml:mi> <mml:mrow> <mml:mn>2</mml:mn> <mml:mi>g</mml:mi> </mml:mrow> </mml:msub> </mml:math> electrons. We find its origin to be the angular dependence in electronic momentum imposed by the kinetic term on the degenerate <?CDATA $j = 3/2$?> <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML overflow=scroll> <mml:mi>j</mml:mi> <mml:mo>=</mml:mo> <mml:mn>3</mml:mn> <mml:mrow> <mml:mo>/</mml:mo> </mml:mrow> <mml:mn>2</mml:mn> </mml:math> manifold. A comparison between the toy model and ab initio results indicates that additional symmetry allowed terms beyond odd-parity spin-conserving inter-orbital hopping processes are needed to describe the Rashba-like polar interaction between the electrons and the soft FE mode." @default.
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- W4313591983 date "2023-01-01" @default.
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- W4313591983 title "Anisotropic Rashba coupling to polar modes in KTaO<sub>3</sub>" @default.
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- W4313591983 doi "https://doi.org/10.1088/2515-7639/acb017" @default.
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