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• W4313593021 startingPage "927" @default.
• W4313593021 abstract "Catalytic transfer hydrogenation of chemically captured CO2 toward MeOH production utilizing ethylene glycol as the hydride donor has been established under mild reaction conditions by employing a Ru(II)–CNN pincer catalyst (CNN = CNHC^Npyridine^Nbenzimidazole tridentate ligand) and a tertiary amine tetramethylethylenediamine (TMEDA). Through a cooperative action with ethylene glycol, TMEDA was found to be the most effective tertiary amine in this integrated CO2 capture/conversion protocol to achieve as high as 64% of MeOH yield and up to 112 catalytic turnovers. Dilute CO2 stream (10% in N2) could also be utilized in this integrated protocol to provide ∼70% yield of MeOH. Involvement of Ru–H active species in the process, generated from the reaction of the catalyst with ethylene glycol, was traced via a spectroscopic investigation. Considering that ethylene glycol can be produced from a renewable bioresource (e.g., nonfood biomass), the developed CO2-to-MeOH transfer hydrogenation protocol integrated with a prior efficient CO2-capturing process represents a prospective approach complementary to the existing catalytic hydrogenation platforms which typically use fossil-derived H2 gas under a high pressure setup." @default.
• W4313593021 created "2023-01-06" @default.
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• W4313593021 date "2023-01-04" @default.
• W4313593021 modified "2023-10-18" @default.
• W4313593021 title "Integrated CO₂ Capture and Conversion to Methanol Leveraged by the Transfer Hydrogenation Approach" @default.
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• W4313593021 doi "https://doi.org/10.1021/acscatal.2c05302" @default.
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