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• W4313593194 endingPage "119574" @default.
• W4313593194 startingPage "119574" @default.
• W4313593194 abstract "In this study, manganese oxide (MnO) dispersed on CN (Mn-nCN) was fabricated as a catalyst in heterogeneous catalytic ozonation (HCO), achieving excellent catalytic performance on refractory organic pollutant degradation via the synergistic effects between MnO and CN. The study demonstrated that the C–N−Mn and C−O−Mn bonds constructed in the catalyst linking MnO and CN created the synergistic effects which could overcome typical problems, such as metal leaching etc. The C−N−Mn and C−O−Mn bonds could promote electron transfer from cation-π reactions to form electron-rich Mn(II) sites and electron-poor CN sites. The electron-rich Mn(II) sites as active sites supplied electrons to ozone which then further evolved into reactive oxygen species (ROS). The electron-poor CN sites captured electrons from the pollutant intermediate radicals to electron-rich Mn(II) sites via cation-π reactions with the help of C−N−Mn and C−O−Mn bonds, which promote the redox reactions of Mn. The surface hydroxyl groups also participated in ozone decomposition and ROS production. Additionally, •OH was the dominant ROS of the Mn-nCN HCO processes. This study presents the excellent HCO performance of Mn-nCN, as well as provides views on the electron transfer route between the catalyst, pollutant and ozone, which is crucial for the design of the catalyst." @default.
• W4313593194 created "2023-01-06" @default.
• W4313593194 creator A5018434228 @default.
• W4313593194 creator A5025729375 @default.
• W4313593194 creator A5026177093 @default.
• W4313593194 creator A5029005365 @default.
• W4313593194 creator A5037584456 @default.
• W4313593194 creator A5046880150 @default.
• W4313593194 creator A5047920896 @default.
• W4313593194 creator A5053944161 @default.
• W4313593194 creator A5067279934 @default.
• W4313593194 creator A5070351769 @default.
• W4313593194 date "2023-02-01" @default.
• W4313593194 modified "2023-10-11" @default.
• W4313593194 title "Electron transfer enhancing the Mn(II)/Mn(III) cycle in MnO/CN towards catalytic ozonation of atrazine via a synergistic effect between MnO and CN" @default.
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