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- W4313593718 abstract "The periodical distribution of N and C atoms in the carbon nitride skeleton results in intrinsically insufficient light absorption and serious carrier recombination. Herein, an efficient two-step cystine-mediated strategy was developed to alter the structure symmetry of C3N4 via the introduction of alkyl groups and nitrogen vacancies. The experimental analysis and theoretical calculation confirm that the formation of alkyl groups and nitrogen vacancies can modulate band structure and activate n-π* electron transition. Especially, the charge density in CN-25CYS is redistributed with spatial separation of oxidation and reduction sites, suppressing photogenerated charge recombination effectively. Therefore, the distorted carbon nitride (CN-25CYS) exhibits 9.6-times and 15.6-times higher photoreaction rates in hydrogen production and RhB degradation than the pristine one (CN-0CYS), respectively." @default.
- W4313593718 created "2023-01-06" @default.
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- W4313593718 date "2023-02-01" @default.
- W4313593718 modified "2023-10-15" @default.
- W4313593718 title "Atomic symmetry alteration in carbon nitride to modulate charge distribution for efficient photocatalysis" @default.
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- W4313593718 doi "https://doi.org/10.1016/j.jcat.2023.01.003" @default.
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