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• W4313594757 endingPage "141264" @default.
• W4313594757 startingPage "141264" @default.
• W4313594757 abstract "“Shuttle effect” is a serious obstacle in the development of high-performance lithium-sulfur batteries and modified separator is considered an effective strategy to prevent the shuttle effect of soluble polysulfides (LiPSs). Herein, we demonstrate a modified polypropylene (PP) separator composed of nitrogen-doped carbon coated LiFePO4 (NC-LFP), Ketjen black carbon (KB) and polyvinylidene fluoride (PVDF) (NC-LFP interlayer), which can improve adsorption and catalytic conversion toward LiPSs. The analysis shows that NC-LFP interlayer could effectively adsorb LiPSs and therefore suppress its shuttle effects due to the FeNC functional groups in the nitrogen-doped carbon coated on LFP polar particles. The DFT analysis and the electrochemical performance test demonstrate the FeNC functional groups in NC-LFP interlayer provide lower activation barrier for catalytic conversion reaction of LiPSs to Li2S and vice versa. The coin cells with NC-LFP modified separator exhibit an initial discharge specific capacity of 907 mAh/g at 1C. After 500 cycles, the specific capacity is 702 mAh/g with a retention rate of 79.5 %. Moreover, at 8C rate, the discharge-specific capacity of 667.5 mAh/g is achieved. The use of NC-LFP interlayer modified separators realizes lithium-sulfur batteries with long-cycle life and high-rate performance, providing an emerging strategy for high-performance Li-S batteries." @default.
• W4313594757 created "2023-01-06" @default.
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• W4313594757 date "2023-02-01" @default.
• W4313594757 modified "2023-10-18" @default.
• W4313594757 title "Synergetic effects of Fe N C and LiFePO4 in modified separator on improved adsorption and catalytic conversion reaction of soluble LiPSs for Lithium-sulfur batteries" @default.
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• W4313594757 doi "https://doi.org/10.1016/j.cej.2022.141264" @default.
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