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- W4313596154 abstract "Abstract The development of earth‐abundant and non‐noble based metal catalysts for electrochemical nitrogen reduction towards sustainable ammonia production from N 2 and H 2 O in the ambient atmosphere holds immense potential in realizing an alternate route to energy‐intensive Haber‐Bosch process. Herein, we have employed highly conductive MoO 2 synthesized by hydrothermal route as an electrocatalyst for ammonia generation. The MoO 2 catalyst was employed for electrochemical nitrogen reduction in N 2 saturated 0.1 m HCl electrolyte in a two‐compartment cell. Ammonia yield rate of 2.30 μg h −1 mg −1 cat and 2.40 % Faradaic efficiency has been obtained at a potential of −0.3 V vs. RHE. The MoO 2 catalyst is selective for ammonia generation without any hydrazine formation. The metallic nature of MoO 2 catalyst assists in achieving comparable activity for the electrochemical nitrogen reduction. The above catalyst has the potential for providing better ammonia yield rate by combining or doping with other active elements." @default.
- W4313596154 created "2023-01-06" @default.
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- W4313596154 date "2023-01-04" @default.
- W4313596154 modified "2023-10-12" @default.
- W4313596154 title "Metallic MoO<sub>2</sub> as a Highly Selective Catalyst for Electrochemical Nitrogen Fixation to Ammonia under Ambient Conditions" @default.
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- W4313596154 doi "https://doi.org/10.1002/slct.202203344" @default.
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