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- W4313596520 abstract "Rational designing of efficient bifunctional oxygen electrocatalysts is significantly important but rather challenging for rechargeable zinc-air batteries. Herein, a novel high-performance bifunctional oxygen electrocatalyst for rechargeable zinc–air batteries are constructed based on bimetal [email protected] encapsulated in in situ grown N,S-doped graphitic carbon framework with within a porous three-dimensional (3D) structure. The final catalyst shows a high half-wave potential of 0.89 V for oxygen reduction reaction, and a low operating overpotential of 0.38 V to achieve a 10 mA cm−2 current density for oxygen evolution reaction. The physical characterizations reveal that a strong synergetic coupling between bimetal [email protected] and S dopant can effectively increase the active sites, meanwhile achieve a rational manipulation of the active site configuration toward a favorable electronic structure. Impressively, the assembled zinc–air batteries using liquid electrolytes and the all-solid-state batteries with this catalyst exhibit excellent charging–discharging performance, long lifetime, and high flexibility." @default.
- W4313596520 created "2023-01-06" @default.
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- W4313596520 date "2023-04-01" @default.
- W4313596520 modified "2023-10-03" @default.
- W4313596520 title "N, S heteroatom co-doped carbon-based materials carrying Mn and Co atoms as bifunctional catalysts for stable rechargeable zinc-air batteries" @default.
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- W4313596520 doi "https://doi.org/10.1016/j.jallcom.2023.168756" @default.
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