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- W4313640057 abstract "In this work, two donor–acceptor linear conjugated polymers were designed and synthesized based on thianthrene-5,5,10,10-tetraoxide (TTO) as the acceptor unit, benzo[1,2-b:4,5-b']dithiophene derivative (Py1) and thiophene (Py2) as the donor units, respectively. The Py1/Py2 composite was prepared by physical ball milling of the two polymers in a mixture, which was further treated with a N-methyl-2-pyrrolidone (NMP)-assisted sonication treatment, and the obtained catalyst was named N-Py1/Py2. Compared with the single polymer or Py1/Py2, the FTIR characteristic peaks of O=S=O have a red shift for N-Py1/Py2, accompanied by a profound change in morphology. Furthermore, N-Py1/Py2 has a broader light response and more efficient separation and transport of charge carriers, and as a result it exhibits a higher photocatalytic hydrogen evolution rate (26.5 mmol g-1 h−1) without the involvement of any co-catalyst than Py1/Py2 catalyst (3.56 mmol g-1 h−1). The underlying mechanism for the enhanced photocatalytic activity by the sonication treatment in NMP is discussed based both on experimental and theoretical calculation data." @default.
- W4313640057 created "2023-01-07" @default.
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- W4313640057 date "2023-04-01" @default.
- W4313640057 modified "2023-09-30" @default.
- W4313640057 title "Enhanced photocatalytic hydrogen evolution activity of co-catalyst free S-scheme polymer heterojunctions via ultrasonic assisted reorganization in solvent" @default.
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- W4313640057 doi "https://doi.org/10.1016/j.jcis.2023.01.016" @default.
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