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• W4313650629 abstract "Phase equilibrium (temperature–composition) relations of the tetra-n-butylphosphonium trifluoroacetate (TBP-TFA) + water binary system including solid (semiclathrate hydrate, SCH)-liquid equilibria and liquid-liquid equilibria were investigated. Phase diagram of TBP-TFA SCH exhibited peritectic behavior. The maximum decomposition temperature (peritectic temperature) of TBP-TFA SCH at atmospheric pressure were 275.9 ± 0.1 K. The stoichiometric composition of TBP-TFA SCH was located at the mole fraction of 0.027 ± 0.002. The decomposition enthalpy of TBP-TFA SCH was 199 ± 2 J/g. At temperatures above the lower critical solution temperature (LCST), the liquid-liquid phase separation appeared. Interestingly, the composition at the LCST was 0.026 ± 0.002, which is very similar to the stoichiometric composition of TBP-TFA SCH. It implies that both cluster-based solution structures are similar." @default.
• W4313650629 created "2023-01-07" @default.
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• W4313650629 date "2023-04-01" @default.
• W4313650629 modified "2023-09-24" @default.
• W4313650629 title "Peritectic phase behavior of tetra-n-butylphosphonium trifluoroacetate semiclathrate hydrate" @default.
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• W4313650629 doi "https://doi.org/10.1016/j.fluid.2023.113727" @default.
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