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- W4313887547 abstract "Cyclic polymers bearing various backbones are selectively synthesized by means of non-stoichiometric Suzuki-Miyaura polycondensation of 1.0 equivalent of diboronate monomers containing carbon–carbon double bond (C=C), ester, ether, and carbonate linkages with 1.3 equivalents of meta- or para-dibromophenylene in the presence of t-Bu3PPd G2 precatalyst and CsF/18-crown-6 as a base. The molecular weight of the cyclic polymers increases with increasing monomer concentration. The obtained polymer containing C=C is cyclic even in the high-molecular-weight region, as confirmed by end-group analysis after degradative cross-metathesis reaction of the obtained polymer with an excess of an olefinic small molecule. This non-stoichiometric A2 + B2 Suzuki-Miyaura polycondensation is expected to be a powerful tool for the synthesis of cyclic polymers containing various functional groups in the backbone." @default.
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- W4313887547 date "2023-02-01" @default.
- W4313887547 modified "2023-10-16" @default.
- W4313887547 title "Synthesis of cyclic polymers containing various backbones by means of non-stoichiometric Suzuki-Miyaura polycondensation through intramolecular catalyst transfer" @default.
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- W4313887547 doi "https://doi.org/10.1016/j.eurpolymj.2023.111828" @default.
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