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• W4313907265 abstract "The nitrogen-deficient graphitic carbon nitride (g-C3 N4 ) has been prepared, a new excited state absorption (ESA) up-conversion mode is discovered, which is directly induced by structural defects, showing distinct chemical characteristics from those based on lanthanide ions and triplet states chromophores. The abundant N2C vacancies in g-C3 N4 nanosheets work as the crucial intermediate excitation states, which lead to g-C3 N4 upconverted emitting at the wavelength of 436 nm excited by the light with the wavelength of 800 nm. This process is proven to proceed via a two-photon involved ESA mode with a breakthrough quantum efficiency of 0.64 %. Further, we combine N2C vacancies enriched g-C3 N4 with In2 S3 and CdS, and successfully achieved an infrared light driven photocatalytic reactions. These findings offered a new family of up-conversion materials; more semiconductors with various structural defects are potential complementary members." @default.
• W4313907265 created "2023-01-10" @default.
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• W4313907265 date "2023-01-24" @default.
• W4313907265 modified "2023-10-15" @default.
• W4313907265 title "Exited State Absorption Upconversion Induced by Structural Defects for Photocatalysis with a Breakthrough Efficiency" @default.
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• W4313907265 doi "https://doi.org/10.1002/anie.202219214" @default.
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